含PEPA基团苯并噁嗪的合成与性能
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河南省教育厅科技攻关项目(2009A150002);河南省科技厅重点攻关项目(092102210210)


Synthesis and properties of PEPA-based benzoxazine
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    摘要:

    以水杨醛,对氨基酚和PEPA的衍生物为原料合成了含笼型磷酸酯结构的苯并噁嗪单体(PEPA-Bz),用FT-IR和1H NMR进行了表征。PEPA-Bz均聚物热失重分析(TGA)结果表明该聚苯并噁嗪具有较好的热稳定性和成炭性能,起始热分解温度235℃,700℃时残炭53%,氧指数达到38.7。采用FT-IR和TGA分别研究了PEPA-Bz与Ba的开环共聚行为及共聚物的热性能。结果表明,含PEPA-Bz苯并噁嗪共聚物的阻燃性和成炭性明显优于不含PEPA-Bz的双酚A型苯并噁嗪树脂。

    Abstract:

    A PEPA-containing benzoxazine (PEPA-Bz) was synthesized from phenol, aniline and PEPA derivative. The structure of target compound was confirmed by fourier transform infrared spectroscopy (FT-IR) and 1H nuclear magnetic resonance spectroscopy (1H NMR). And the properties of its homopolymer and its copolymer with bisphenol-based benzoxazine(Ba) were investigated. Thermal gravimetric analysis (TGA) showed that PEPA-containing polybenzoxazine has good thermal stability and char formation. The temperature at 5% weight loss is 235℃, the char yield ratio is 53% at 700℃and the LOI is 38.7. FT-IR and TGA were utilized to investigate the ring-opening copolymerization behavior of PEPA-Bz and Ba and their thermal properties, respectively. The results shows that the Flame retardant properties and char yield of the copolymer were both better than the homopolymer of Ba.

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房晓敏,胡永佳,张璞,徐元清,丁涛,任艳蓉.含PEPA基团苯并噁嗪的合成与性能[J].精细化工,2011,28(11):

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  • 收稿日期:2011-07-08
  • 最后修改日期:2011-09-15
  • 录用日期:2011-09-16
  • 在线发布日期: 2011-10-25
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