新型聚羧酸系混凝土减水剂的研究(Ⅰ)——酯化大单体的制备与表征
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Study of A New Polycarboxylate Type Superplasticizers (Ⅰ)——Preparation and Characterization of Macromonomer
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    摘要:

    通过衣康酸与聚乙二醇的酯化反应,制备出了一种可用于合成聚羧酸系减水剂的大分子单体。用正交实验研究了反应条件对酯化反应的影响,确定了最佳的酯化反应条件为n衣康酸:n聚乙二醇-1000为1:1.1,催化剂用量为聚乙二醇-1000质量的4%,反应温度100 ℃,反应时间6 h,带水剂用量为聚乙二醇-1000质量的30%,阻聚剂用量为衣康酸质量的2%。在该条件下单酯化率可达到98.3%。并通过红外光谱、氢核磁共振谱对大分子单体进行了表征,结果表明得到了衣康酸聚乙二醇酯大单体。

    Abstract:

    A new intermediate macromonomer for polycarboxylate type superplasticizers was prepared by esterification of itaconic acid and polyethylene glycol. The conditions of the esterification were investigated by orthogonal experiment. The optimum conditions were obtained as follows: the molar ratio of itaconic acid to polyethylene glycol is 1:1.1; the amount of catalyst is 4% according to the mass of polyethylene glycol; the reaction temperature is 100℃; the reaction time is 6h; the amount of water-carrying agent is 30% according to the mass of polyethylene glycol and the amount of polymerization inhibitor is 2% according to the mass of itaconic acid. Under the optimum conditions, the percentage of esterification is as high as 98.3%. The macromonomer was characterized by FTIR and 1H-NMR. The result indicated that the macromonomer, the itaconic acid polyethylene glycol ester, was obtained.

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苏瑜,庞浩,王斌,蒋冰艳,张磊,廖兵.新型聚羧酸系混凝土减水剂的研究(Ⅰ)——酯化大单体的制备与表征[J].精细化工,2012,29(2):

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  • 收稿日期:2011-11-05
  • 最后修改日期:2011-11-05
  • 录用日期:2011-11-21
  • 在线发布日期: 2012-01-09
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