RAFT聚合制备温敏性含糖共聚物
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O631;TQ316

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纤维材料改性国家重点实验室开放课题(LK0908)


Synthesis of Thermosensitive Glycopolymer by RAFT
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    摘要:

    采用酶促法合成了含糖单体6-O-乙烯基己二酸-D-吡喃型葡萄糖酯(OVAG),使用可逆加成链断裂转移自由基聚合法(RAFT聚合)将N-异丙基丙烯酰胺(NIPAAm)和OVAG共聚,制备分散度(PDI)低且具有温度敏感性的含糖高聚物Poly(NIPAAm-co-OVAG)。用1H NMR,傅里叶变换红外光谱(FTIR),凝胶渗透色谱(GPC)对聚合物进行了表征。通过透射电子显微镜(TEM)发现自组装形成的聚合物胶束结构规整且粒径均匀。通过紫外-可见光谱对聚合物温敏性检查表明,共聚物的低临界溶解温度(LCST)可以通过共聚单体的比例进行调控。当NIPAAm与OVAG的物质的量之比为14:1时,共聚物的LCST值为36 oC,在人体温度下可以形成纳米胶束,在药物载体方面拥有广阔前景。

    Abstract:

    The glycomonomer 6-O-vinyladipoyl-D-glucopyranose (OVAG) was synthesized by lipase catalyzed transesterification of divinyladipate with D-glucopyranose. Poly(NIPAAm-co-OVAG) with narrow polydispersity (PDI) and thermosensitivity was prepared via Reversible Addition-Fragmentation Chain Transfer (RAFT) polymerization. The Poly(NIPAAm-co-OVAG) was characterized by 1H NMR, FTIR and gel permeation chromatography (GPC). Measurement by transmission electron microscopy (TEM) revealed that Poly(NIPAAm-co-OVAG) was able to self-assemble into nano micelle with well-defined structure and uniform size in aqueous solution. The characterization of UV-visible spectroscopy showed that the low critical solution temperature (LSCT) can be controlled by the molar ratio of monomers. When the molar ratio of NIPAAm and OVAG was 14:1, the LCST of Poly(NIPAAm-co-OVAG) was 36oC in aqueous solution, which can form nano micelle in the human body environment and has great potential in drug carrier.

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孙衎,石萌,巫寒冰,朱燕平,聂华丽,权静,朱利民. RAFT聚合制备温敏性含糖共聚物[J].精细化工,2013,30(12):

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  • 收稿日期:2013-06-27
  • 最后修改日期:2013-08-20
  • 录用日期:2013-08-21
  • 在线发布日期: 2013-12-04
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