Page 80 - 《精细化工》2023年第4期
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g766g ㏳ࡃጒ FINE CHEMICALS す 40 ࢤ
ₑ喑ज̻ڤᰶхᐯ⩢ࡃ႓ᕔ㘪⮱ᄩ⩢➖䉕ฺव [30] ȡ H 2 O喎ݣิγ܊㘣⩢㼐䉕ȡDMSO Ӱ䔈γ PVA ⮱܊
⢸䯲ैぶ [31] В CNF ͧ܊㘣⩢㼐䉕⮱㏠ㆠ᫆喑ᩜᦾ 㘣ࡃ喑㔹 CNF ݆҉ͧڣ͚⮱㏠ㆠ᫆喑ᓄݝ⮱܊㘣
ᄩ⩢ധ䉕㑾㐉ᝃ᭜Ⱑᣒٲᒀ俕᳣ӈ߈႓ᩜᦾহ ⩢㼐䉕ڤᰶᲮ倅⮱䴔ᕔ喑៶ѥᏁअ>600%⮱हᬣᏁ߈
ӈ㑾㐉㐀Ჱ喑ݣิܧڤᰶхᐯ⩢ࡃ႓হ߈႓ᕔ㘪⮱ 䓫ݝγ 2.1 MPaȡₑใ喑CNF ⮱ႅౕҬ PVA 俕᳣ᒏ
܊㘣⩢㼐䉕ȡCHEN ぶ [32] ݣิ⮱㏠ㆠ㏑㐡㉍܊㘣 γᰡ็ᅯ⁎⮱็ႁ㐀Ჱȡ㐀㶕ᬻ喑⌨ߍγ PVA
䕇䓴倅㏠ㆠ㏑㐡㉍⮱䪬ᒱ℁ᰶ᩵ౝࡴγ܊㘣⮱ 䉕䛼 4%⮱ CNF ऻ喑⩢㼐䉕⮱⻨ၽ⩢ᄩ⢴䒰㏜ PVA
߈႓ᕔ㘪喑ᰡ๔⮱䪬ᒱ℁ΌᘼঠⱭ㐆܊㘣ፓᲒᰡ͝ ܊㘣ࡴγ 2 Ժ喑Ꭳ́ DMSO ⮱ႅౕҬ䄒܊㘣⩢㼐
ჹ⮱ႁ䯆㐀Ჱࣷ℁㶕䲏⼜喑㘪ͧᄩ⩢➖䉕ӈᰡ็ 䉕जВౕ䊲ѻ⍖⣜ධ̸ࣾᡒ҉⩕ȡSONG ぶ [36] ݣิ
⮱ฺवѺ◦ȡₑใ喑ZHANG ぶ [33] 䔅ࣾ⣝喑㏠ㆠ㏑ ⮱܊㘣⩢㼐䉕ӊ䲍ڲ䘕㖇Άι䚴⮱ᴁᕔ䨫⃢̻㏠ㆠ
㐡㉍⮱ႅౕ㘪์Ӱ䔈㏑㐡㉍䨫䬡Ⱕο㑍㐂হ䔋 ᱕䉕㏑㐡㉍喍LCNF喎俕᳣⮱㉔ჳϑ㏴㑾㐉㐀ᲱҬ࠲
ᣒ喑ᰶ᩵㕄᪐γใ⩹Ꮑ߈喑ᑧγ܊㘣߈႓ᕔ㘪ȡ ᠙☚߈႓Ƞ߈႓ࣷ⩢ࡃ႓ぶ็䲏ᕔ㘪䘪ᰶγ᭫㦄
㔹喑ݣิ⮱܊㘣⩢㼐䉕ᑧᏓᬻ᭫倅λ̭㝙ⴠ⇦ ࡴȡMO ぶ [37] В CNF ͧ俕᳣喑[2-(⩟ധ͆☜䚝ധ
ധ㖇व➖܊㘣ȡ ⅔ധ)Άധ]ι⩟ധ-(3-⸧䚥͆ധ)⅏⅔ࡃ䨢ͧࢂҀ喑ᑂ
CNF ̺ϲ҉ͧ㏠ㆠ᫆ᑧγ܊㘣⩢㼐䉕⮱ᑧ ࣾ㜗⩞ധ㖇ववγ͑ᕔ⻨ၽಸ⸧ധ⩉㤉ⷞࢂҀᲒ
Ꮣ̻䴔ᕔ喑䔅䕇䓴⅏䩛̻ڣЃ倅ܳၽ䨫㑍㐂ᒏ㑾 व܊㘣⩢㼐䉕ȡ⩞λ͑ᕔ⻨ၽധఏহⅡܳၽ䬡
⟣㐀ᲱВ䔈̭ₒᑧ܊㘣⩢㼐䉕⮱߈႓ᕔ㘪ȡCHEN ⮱ᑧ䲆⩢Ⱕο҉⩕喑ፓᰶₐ䉌⩢㢤⮱͑ᕔ⻨ၽಸ⮱
ぶ [34] ݣิγक़䨹⯽⮱ⶩϑ㖁㖇Ά☜䚴喍PVA喎/㏠ ⩢㼐䉕ͧ܊㘣ӈγхᐯ⮱ԊⅡᕔ㘪喑㔹 CNF 俕᳣
ㆠ㏑㐡㉍܊㘣⩢㼐䉕喍B-PVA/CNF喎喍ఫ 1喎ȡ 㼐۠γ͑ᕔ⻨ၽ㖇व➖⮱㘳ᕔ䬛䷅喑ϻ㔹Ԋ䃮ڣ㏱
㷲⮱⩢̺чბใ⋟Ⱕ㧥ࣾᝃใ߈ϔ⩌⮱ᑜៅᒞ
৺䪬Ͳ⽠Ⴧጒ҉⮱㘪߈ȡ
CNF ڤᰶ䒰๔⮱䪬ᒱ℁喑̻๔䘕ܳᄩ⩢㖇व➖
ฺवᬣοⰥ㑍㐂㘪ᒏࣹ㑾㐉㐀Ჱ⮱܊㘣⩢㼐䉕喑
CNF 㘪์ٲᒀᑧҀВ倅ڣᱧᷝᑧᏓহ⻨ၽ⩢ᄩ
⢴ȡGE ぶ [38] ౕ CNF হ LiCl ⮱ႅ̸ౕ喑䕇䓴͆☜䚝
㘧喍AM喎̭ₒ㜗㖇ववγࣹ㑾㐉܊㘣喍ఫ 2喎ȡ
CNF ̻㖇͆☜䚝㘧喍PAM喎䬡ᒏ⅏䩛҉⩕হܳ
ၽ䨫䬡㑍㐂喑㘪ᰶ᩵㕄᪐܊㘣⮱ใߍᏁ߈喑䉸ε܊
㘣㞜ສ⮱䴔ᕔȠ៶ѥᕔহࢸ㑖ᕔȡᒀ LiCl ⮱䉕䛼⊀
Ꮣܳݘͧ 100Ƞ300 হ 500 g/L ᬣ喑ݣิγ̭㈨݄
PAM/CNF/LiCl ܊㘣喑ܳݘ䃝ͧ PAM/CNF/LiCl 10%Ƞ
PAM/CNF/LiCl 30%হ PAM/CNF/LiCl 50%喑ڣ͚喑
PAM/CNF/LiCl 50%܊㘣҉ͧ⩢㼐䉕㏱㷲⮱䊲㏔⩢
ღகౕѻ⍖У̸ڤᰶ⽠Ⴧ⮱⩢ࡃ႓ᕔ㘪হ倅䓫
748%⮱ᐣᆂ ᕔ喑ह ᬣ⻨ ၽ⩢ᄩ ⢴ౕ –40 Ď倅䓫
2.25 S/mȡWANG ぶ [39] ݣิγ̭㖇͆☜䚝㘧-叱࣌
㘣ᣒ㖇व➖ฺव CNF喑ڣ㘪์ౕ䨹⯽⏣⋟͚㏱㷲
ఫ 1 B-PVA/CNF ܊㘣⩢㼐䉕ݣิࣷᱧ⤳ᘼఫ喍a~b喎喠
܊㘣⩢㼐䉕៶ѥ̻㜗ԛฺ➖ఫ喍c喎 [34] ࣹ㑾㐉㐀Ჱ܊㘣⩢㼐䉕ȡCNF ҉ͧӈᓛႁ㑾㐉
Fig. 1 Schematic diagram of preparation and mechanism 㐀Ჱ⮱ϟⅡᕔ俕᳣喑㘪์ٲᒀᑧҀВ倅܊㘣⩢
of B-PVA/CNF gel electrolyte (a~b); Stretching and 㼐䉕⮱ᱧᷝᑧᏓহ⻨ၽ⩢ᄩ⢴喑ᰭ㏵⩢㼐䉕⻨ၽ⩢
self-healing physical diagram of gel electrolyte
(c) [34] ᄩ⢴䓫ݝγ 28.8 mS/cm喑हᬣᏁअࡴγ 4 Ժ喑ധ
λ䄒⩢㼐䉕㏱㷲⮱䨹⩢ጟ㏼㘪ͧᴁᕔज⾬ᝡ⩢ၽ
PVA হ CNF 䬡ज䕇䓴ⶩ⣝γߕᔮज䔳 䃫ิ䔈㵹ӈ⩢ȡ
ϑ㖁喑ᰭ㏵㣤ᓄ⮱܊㘣⩢㼐䉕᠒ᰶхᐯ⮱叼ᑦᕔȠ 㐩̷喑⩕㏠ㆠᅧᏓ⮱ CNF ݣิ⮱܊㘣⩢㼐䉕ڤ
㞜ສ⮱叼㐀ᕔ㘪হᲮᑧ⮱㜗ᘵᕔ㘪喑Ꭳ́ڤᰶ ᰶ͝ჹȠ㜡ჳ⮱ႁ䯆㐀Ჱ喑㘪䔈̭ₒ倅ڣ䴔ᕔࣷ
18.1 mS/cm ⮱倅⻨ၽ⩢ᄩ⢴喑ᰭ㏵㏱㷲जៅऍᑜ ⻨ၽэᄩᕔ㘪ȡओใ喑㏠ㆠ㏑㐡㉍㘪̻ڣЃᄩ⩢㖇
ᰟВࣷज㜗ᘵव⮱䊲㏔⩢ღகȡYE ぶ [35] ᄳ PVA ̻ व➖ฺवϑ㖁㔹̺ϔ⩌ᢿ喑ϻ㔹䉸ε܊㘣⩢㼐䉕
CNF ⌤वऻ䕇䓴ᑂڒι⩟ധχⵉⅡ⏣⋟喍DMSO/ 㜗ᘵवぶᕔ㘪ȡ㏑㐡㉍㏠ㆠҀ㈨Ⱕ䒰⏣㼐Ҁ㈨ⵁ⾣